Hidden Magnetic States Emergent Under Electric Field, In A Room Temperature Composite Magnetoelectric Multiferroic
Clarkson, J. D. et al. ; The ability to control a magnetic phase with an electric field is of great current interest for a variety of low power electronics in which the magnetic state is used either for information storage or logic operations. Over the past several years, there has been a considerable amount of research on pathways to control the direction of magnetization with an electric field. More recently, an alternative pathway involving the change of the magnetic state (ferromagnet to antiferromagnet) has been proposed. In this paper, we demonstrate electric field control of the Anomalous Hall Transport in a metamagnetic FeRh thin film, accompanying an antiferromagnet (AFM) to ferromagnet (FM) phase transition. This approach provides us with a pathway to "hide" or "reveal" a given ferromagnetic region at zero magnetic field. By converting the AFM phase into the FM phase, the stray field, and hence sensitivity to external fields, is decreased or eliminated. Using detailed structural analyses of FeRh films of varying crystalline quality and chemical order, we relate the direct nanoscale origins of this memory effect to site disorder as well as variations of the net magnetic anisotropy of FM nuclei. Our work opens pathways toward a new generation of antiferromagnetic – ferromagnetic interactions for spintronics. ; Te work at Berkeley was supported in part by FAME, one of six centers of STARnet, a Semiconductor Research Corporation program sponsored by MARCO and DARPA was supported by the SRC-FAME program. Financial support by the Spanish Government (Project MAT2014-56063-C2-1-R, MAT2015-73839-JIN, MAT2017- 85232-R and associated FEDER) and Generalitat de Catalunya (2014 SGR 734) is acknowledged. ICMAB-CSIC authors acknowledge fnancial support from the Spanish Ministry of Economy and Competitiveness, through the "Severo Ochoa" Programme for Centres of Excellence in R&D (SEV- 2015-0496). IF acknowledges Juan de la Cierva – Incorporación postdoctoral fellowship (IJCI-2014-19102) from the Spanish Ministry of Economy and Competitiveness of Spanish Government. XMCD-PEEM experiments were performed at CIRCE beamline at ALBA Synchrotron with the acknowledged collaboration of ALBA staf. Partial fnancial support from the 2014-Consolidator Grant "SPIN-PORICS" (Grant Agreement nº 648454) from the European Research Council is acknowledged. XM acknowledges support from the Grant Agency of the Czech Republic Grant no. 14-37427. Work at ORNL was sponsored by the Laboratory Directed Research and Development (LDRD) Programs of ORNL managed by UT-Battelle, LLC. Work at CSUN was supported by NSF under Grant No. 1205734, NSF Partnerships for Research and Education in Materials (PREM), and by NSF under Grant No. 1160504 NSF Nanosystems Engineering Research Center for Translational Applications of Nanoscale Multiferroic Systems (TANMS). ; Peer reviewed