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6 pags., 5 figs., 1 tab. ; There is sparse direct experimental evidence that atomic nuclei can exhibit stable "pear" shapes arising from strong octupole correlations. In order to investigate the nature of octupole collectivity in radium isotopes, electric octupole (E3) matrix elements have been determined for transitions in Ra222,228 nuclei using the method of sub-barrier, multistep Coulomb excitation. Beams of the radioactive radium isotopes were provided by the HIE-ISOLDE facility at CERN. The observed pattern of E3 matrix elements for different nuclear transitions is explained by describing Ra222 as pear shaped with stable octupole deformation, while Ra228 behaves like an octupole vibrator. ; The support of the ISOLDE Collaboration and technical teams is acknowledged. This work was supported by the following Research Councils and Grants: Science and Technology Facilities Council (UK) Grants No. ST/P004598/1, No. ST/L005808/1, No. ST/ R004056/1; Federal Ministry of Education and Research (Germany) Grants No. 05P18RDCIA, No. 05P15PKCIA, and No. 05P18PKCIA and the "Verbundprojekt 05P2018"; National Science Centre (Poland) Grant No. 2015/18/M/ ST2/00523; European Union's Horizon 2020 Framework research and innovation programme 654002 (ENSAR2); Marie Skłodowska-Curie COFUND Grant (EU-CERN) 665779; Research Foundation Flanders and IAP Belgian Science Policy Office BriX network P7/12 (Belgium); GOA/2015/010 (BOF KU Leuven); RFBR (Russia) Grant No. 17-52-12015; and the Academy of Finland (Finland) Grant No. 307685.

6 pags., 4 fig.s, 1 tab. -- Open Access funded by Creative Commons Atribution Licence 4.0 ; There is a large body of evidence that atomic nuclei can undergo octupole distortion and assume the shape of a pear. This phenomenon is important for measurements of electric-dipole moments of atoms, which would indicate CP violation and hence probe physics beyond the Standard Model of particle physics. Isotopes of both radon and radium have been identified as candidates for such measurements. Here, we observed the low-lying quantum states in Rn and Rn by accelerating beams of these radioactive nuclei. We show that radon isotopes undergo octupole vibrations but do not possess static pear-shapes in their ground states. We conclude that radon atoms provide less favourable conditions for the enhancement of a measurable atomic electric-dipole moment. ; The support of the ISOLDE Collaboration and technical teams is acknowledged. This work was supported by the following Research Councils and Grants: Science and Technology Facilities Council (STFC; UK) grants ST/ P004598/1, ST/L005808/1; Federal Ministry of Education and Research (BMBF; Germany) grants 05P18RDCIA, 05P15PKCIA and 05P18PKCIA and the "Verbundprojekt 05P2018"; National Science Centre (Poland) grant 2015/18/M/ST2/00523; European Union's Horizon 2020 Framework research and innovation programme 654002 (ENSAR2); Marie Skłodowska-Curie COFUND grant (EU-CERN) 665779; Research Foundation Flanders (FWO, Belgium), by GOA/2015/010 (BOF KU Leuven) and the Interuniversity Attraction Poles Programme initiated by the Belgian Science Policy Office (BriX network P7/12); RFBR(Russia) grant 17-52-12015.