Probing the lattice anharmonicity of superconducting YBa2Cu3O7−δ via phonon harmonics
We examine coherent phonons in a strongly driven sample of optimally-doped high temperature superconductor YBa2Cu3O7−δ . We observe a nonlinear lattice response of the 4.5 THz copper-oxygen vibrational mode at high excitation densities, evidenced by the observation of the phonon third harmonic and indicating the mode is strongly anharmonic. In addition, we observe how high-amplitude phonon vibrations modify the position of the electronic charge transfer resonance. Both of these results have important implications for possible phonon-driven nonequilibrium superconductivity ; This project has received funding from the European Research Council (ERC) under the European Union's Horizon 2020 research and innovation programme (Grant agreement No. 758461 and was supported by Spanish MINECO (Severo Ochoa Grants No. SEV-2015-0522 and No. SEV-2015-0496), Ramón y Cajal programme RYC2013-14838, and Fondo Europeo de Desarrollo Regional FIS2015-67898-P (MINECO/FEDER), MAT2014-51778- C2-1-R as well as Fundació Privada Cellex, and CERCA Programme/Generalitat de Catalunya. ; Peer reviewed